The Effect of the Interfacial Exchange Interaction on the Metastability of Magnetic States of Core/Shell Nanoparticles

I. G. Il’yushina, *, L. L. Afremova, and V. N. Kharitonovb

a Department of Theoretical Physics and Intelligent Technologies, Institute of High Technologies and Advanced Materials, Far Eastern Federal University, Vladivostok, 690922 Russia

b Laboratory for Simulation of Physical Processes, Institute of High Technologies and Advanced Materials, Far Eastern Federal University, Vladivostok, 690922 Russia

Correspondence to: *e-mail: iliushin.ig@dvfu.ru

Received 4 October, 2022

Abstract—Within the model of two-phase (core/shell) ellipsoidal nanoparticles, the effects of the interfacial exchange interaction, size, elongation, and orientation of the major axes of the core and shell on the metastability of magnetic states have been simulated. Using the example of ${{{\text{F}}{{{\text{e}}}_{3}}{{{\text{O}}}_{4}}} \mathord{\left/ {\vphantom {{{\text{F}}{{{\text{e}}}_{3}}{{{\text{O}}}_{4}}} {{\text{F}}{{{\text{e}}}_{{2.44}}}{\text{T}}{{{\text{i}}}_{{0.56}}}{{{\text{O}}}_{4}}}}} \right. \kern-0em} {{\text{F}}{{{\text{e}}}_{{2.44}}}{\text{T}}{{{\text{i}}}_{{0.56}}}{{{\text{O}}}_{4}}}}$ nanoparticles, it is shown that the metastability of magnetic states is realized in a limited range of the constant of interfacial exchange interaction between the core and shell, ${{A}_{{{\text{in}}}}}$, and geometric parameters. With an increase in the absolute value of the interfacial exchange interaction constant, $\left| {{{A}_{{{\text{in}}}}}} \right|$, from ${{A}_{{{\text{in}}}}} = 0$ to some finite value, the metastability of magnetic states decreases monotonically from maximum to zero, regardless of the angle between the major axes of the core and the shell.

Keywords: metastability, interfacial exchange interaction, core/shell nanoparticles

DOI: 10.1134/S0031918X22601792